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One-electron oxidation of L2PdII(CH3)2 complexes Ligand effects on production of ethane vs. Pd–C bond homolysis》.pdf
Polyhedron 84 (2014) 44–50 Contents lists available at ScienceDirect Polyhedron journal homepage: www.else /locate/poly II One-electron oxidation of L Pd (CH ) complexes: Ligand effects 2 3 2 on production of ethane vs. Pd–C bond homolysis Michael P. Lanci 1, Bradley A. McKeown, David B. Lao, Karen E. Spettel 2, James M. Mayer ⇑ Department of Chemistry, University of Washington, Box 351700, Seattle, WA 98195-1700, USA a r t i c l e i n f o a b s t r a c t Article history: II Dimethyl palladium(II) complexes with various bi- and tri-dentate ligands, (L )Pd (CH ) , react readily 2 3 2 Received 3 April 2014 + with the one-electron oxidant ferrocenium hexafluorophosphate (Fc ) in acetone-d . These oxidations 6 Accepted 3 June 2014 typically proceed by one of two pathways.
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