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alignment-dependent atomic model for electron transfer in ion-molecule collisionsalignment-dependent原子模型的电子转移离子分子碰撞
Int. J. Mol. Sci. 2002, 3, 132-141
International Journal of
Molecular Sciences
ISSN 1422-0067
© 2002 by MDPI
/ijms/
Alignment-Dependent Atomic Model for Electron Transfer in
Ion-Molecule Collisions
*
C. D. Lin and Ingrid Reiser
J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506
U.S.A.
*Author to whom correspondence should be addressed. E-mail: cdlin@
Received: 23 October 2001/ Accepted: 19 November 2001/ Published: 28 March 2002
Abstract: The alignment-dependent atomic model for treating electron transfer processes in
ion-molecule collisions [Shingal and Lin, Phys. Rev . 1989, A40, 1302] is reviewed. This
model has been applied to collisions between H+ and He2+ with H , and recently also to
2
collisions between He2+ and Ar2+ ions with H2+, where alignment effect is being explored
experimentally.
Keywords: ion-molecule collisions; close-coupling method; alignment effect; ion-ion colli-
sions.
Introduction
Electron captures from atoms or molecules in collisions with ions in the keV to MeV energy region
have been extensively studied over the last few decades. For simple atomic targets with one or two ac-
tive electrons the close-coupling method, based either on atomic orbitals (AO) [1] or molecular orbitals
(MO) [2], has been successfully applied to obtain accurate cross sections fo
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