First-order-Reversal-Curve-Analysis-of-Phase-Transitions-in-Electrochemical-Adsorption：A-New-Experimental-Technique-Suggested-by-Computer-Simulations.pdfVIP

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First-order-Reversal-Curve-Analysis-of-Phase-Transitions-in-Electrochemical-Adsorption：A-New-Experimental-Technique-Suggested-by-Computer-Simulations.pdf

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First-order-Reversal-Curve-Analysis-of-Phase-Transitions-in-Electrochemical-Adsorption：A-New-Experimental-Technique-Suggested-by-Computer-Simulations

First-order Reversal Curve Analysis of Phase Transitions in Electrochemical Adsorption: A New Experimental Technique Suggested by Computer Simulations 1,2 2 1,2,3 I. Abou Hamad , D.T. Robb , P.A. Rikvold 1 Center for Materials Research and Technology and Department of Physics, Florida State University, Tallahassee, FL 32306-4350, USA 2School of Computational Science, Florida State University, Tallahassee, FL 32306-4120, USA 3National High Magnetic Field Laboratory, Tallahassee, FL 32310 July 3, 2006 Abstract The ﬁrst-order reversal curve (FORC) method for analysis of sys- tems undergoing hysteresis is applied to dynamical models of electro- chemical adsorption. In this setting, the method can not only diﬀer- entiate between discontinuous and continuous phase transitions, but can also quite accurately recover equilibrium behavior from dynamic analysis for systems with a continuous phase transition. Discontinu- ous and continuous phase transitions in a two-dimensional lattice-gas model are compared using the FORC method. The FORC diagram for a discontinuous phase transition is characterized by a negative (un- stable) region separating two positive (stable) regions, while such a negative region does not exist for continuous phase transitions. Ex- perimental data for FORC analysis could easily be obtained by simp