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control of mechanical properties of thermoplastic polyurethane elastomers by restriction of crystallization of soft segment热塑性聚氨酯弹性体的力学性能的控制限制软链段的结晶
Materials 2010, 3, 5097-5110; doi:10.3390/ma3125097 OPEN ACCESS materials ISSN 1996-1944 /journal/materials Review Control of Mechanical Properties of Thermoplastic Polyurethane Elastomers by Restriction of Crystallization of Soft Segment Ken Kojio 1,*, Mutsuhisa Furukawa 2, Yoshiteru Nonaka 3 and Sadaharu Nakamura 3 1 Materials Science and Engineering Department, Faculty of Engineering, Nagasaki University, 1-14 Bunkyo-machi, Nagasaki 852-8521, Japan 2 Nagasaki University, 1-14 Bunkyo-machi, Nagasaki 852-8521, Japan; E-Mail: furukawa@nagasaki-u.ac.jp 3 Materials and Science Department, Graduate School of Science and Technology, Nagasaki University, 1-14 Bunkyo-machi, Nagasaki 852-8521, Japan * Author to whom correspondence should be addressed; E-Mail: kojio@nagasaki-u.ac.jp; Tel.: +81-95-819-2652; Fax: +81-95-819-2652. Received: 25 October 2010, in revised form: 19 November 2010 / Accepted: 29 November 2010 / Published : 1 December 2010 Abstract: Mechanical properties of thermoplastic polyurethane elastomers based on either polyether or polycarbonate (PC)-glycols, 4,4’-dipheylmethane diisocyanate (1,1’-methylenebis(4-isocyanatobenzene)), 1,4-butanediol, were controlled by restriction of crystallization of polymer glycols. For the polyether glycol based-polyurethane elastomers (PUEs), poly(oxytetramethylene) glycol (PTMG), and PTMG incorporating dimethyl groups (PTG-X) and methyl side groups (PTG-L) were employed as a polymer glycol. For the PC-glycol, the randomly c
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