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Ac impedance modelling of nickel hydroxide electrodes viewed as mixed protonic-electronic conductors.pdf
ElecrrochnmicaActo, Vol. 41. Nos. 7/S. pp. 1259-1265. 1996
Copyright C 1996 Elmvkr Science Ltd.
Printed in Great Britain. All rights reserved
0013~4686/96 $15.00 + 0.00
0013~4686(95)00446-7
AC IMPEDANCE MODELLING OF NICKEL HYDROXIDE
ELECTRODES VIEWED AS MIXED
PROTONIC-ELECTRONIC CONDUCTORS
V. MANGIER,* A. MBTROT*$and P. WILLMANNt
+ Laboratoire d’Electrochimie et Chimie du Solide, Facultt des Sciences, BP 1039,51687 Reims cedex 2,
France
t CNES, 18 avenue E. Belin, 31055 Toulouse cedex, France
(Received 8 May 1995)
Abstract-Nickel hydroxide electrodes have been studied by nc impedance spectroscopy at rest potential
and during charge or discharge. A transmission line model is proposed based on behaviour similarities
with electrochemical intercalation into graphite. Considering here that protons and electrons react inside
the solid, partial electronic and protonic conductivities of the two p-type phases Ni(OH), and NiOOH in
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